Direct Synthesis of Acetic Acid from CH4-CO2 by a Step-Wise Route over TiO2-supported Co, Pd single and bimetal catalysts
The conversion of CH4 and CO2 into valuable chemical products such as acetic acid is an important subject in the field of C1 chemistry. As it is known, the chemical fixation of CO2 requires consumption of hydrogen while the chemical utilization of CH4 requires oxygen; conversing CH4 and CO2 togather is an ideal reaction to combine oxygenation with reduction. The direct synthesis of acetic acid from CH4 and CO2 is an atomic economic reaction, but it is also thermodynamically unfavorable. Much work has been done to overcome such thermodynamic limitation, among which homogeneous catalytic systems were widely introduced 1-4.
Zhiqin Li Wei Huang Tingdong Zhao
Key Laboratory of Coal Science and Technology, Ministry of Education and Shanxi Province Institute of Coal Chemistry and Engineering, Taiyuan University of Technology, Taiyuan 030024, China
国际会议
第七届中韩清洁能源研讨会(The 7th China-Korea Workshop on Clean Energy Technology)
太原
英文
273-274
2008-06-25（万方平台首次上网日期，不代表论文的发表时间）