Catalytic combustion of methane over supported manganese oxide catalysts
Supported manganese oxide catalysts for methane catalytic combustion were prepared by the incipient wetness impregnation method, and the effects of support (Al2O3, SiO2 and TiO2) and Mn loading were investigated. These catalysts were characterized with N2 adsorption, X-ray diffraction, X-ray photoelectron spectroscopy and temperature-programmed reduction techniques. Methane conversions vary over a large range depending on the supports and Mn loadings, Al2O3 supported 15％ Mn catalyst is found to be the highest activity towards methane oxidation. The existent state of manganese and oxygen species are found to play an important role in catalytic activities of supported manganese catalysts.
Methane catalytic combustion Manganese oxide catalysts Support effect Alumina
Jinyan Hu Wei Chu Muhua Chen Fenfen Qu Limin Shi
Department of Environmental Science and Engineering, Sichuan University, Chengdu 610065, China;Depar Department of Chemical Engineering, Sichuan University, Chengdu 610065, China Department of Environmental Science and Engineering, Sichuan University, Chengdu 610065, China
国际会议
第四届中日化工学术研讨会(The 4th Joint China/Japan Chemical Engineering Symposium)(CJCES)
成都
英文
2007-12-19（万方平台首次上网日期，不代表论文的发表时间）